Cancer Patent

Compositions and methods for treatment of cancer

Cancer Patent Abstract



The present invention concerns compositions and methods for the treatment of disorders characterized by the over-expression of an LIV-1. More specifically, the compositions include DNA and amino acid sequences of an LIV-1, antibodies to an LIV-1, and methods for the treatment of a mammal susceptible to or diagnosed with cancer wherein an LIV-1 is overexpressed.

Cancer Patent Claims
What is claimed is:

1. A method of diagnosing tumor in a mammal, comprising detecting and quantifying the level of expression of a nucleic acid sequence comprising a sequence 100% identical to the sequence from nucleotide 412 to and including nucleotide 477 of SEQ ID NO: 3 or to its fully complementary sequence in a test sample obtained from the mammal, and in a control sample, wherein a higher expression level in the test sample indicates the presence of tumor in the mammal from which the test sample was obtained.

2. The method of claim 1, wherein said test sample is obtained from an individual suspected to have neoplastic cell growth or proliferation.

3. The method of claim 2, wherein the sample is from breast tissue of the mammal.

Cancer Patent Description
FIELD OF THE INVENTION

The present invention concerns compositions and methods for the treatment of disorders characterized by the overexpression of a LIV-1 gene product in tumors. The compositions comprise a nucleic acid, a polypeptide encoded by the nucleic acid, and a compound, preferably an antibody or fragment thereof, that binds to the polypeptide, preferably binding to the extracellular domain of LIV-1 polypeptide.

BACKGROUND OF THE INVENTION

Breast cancer is a common and devastating form of cancer, affecting millions of women per year throughout the world. Many breast tumors are estrogen sensitive and frequently treatable with compounds that interfere with estrogen binding to estrogen receptors (ERs) expressed on the breast tumor tissue. Detecting the level of ER expression and sensitivity to estrogen stimulation is useful for determining that antihormone-type chemotherapy may succeed in a particular patient.

The overexpression of estrogen-inducible genes, pLIV-1 and pLIV2 (also designated pS2), occurs in some breast tumors which also express the estrogen receptor, (Manning D. L. et al. European J. Cancer 29A(10): 1462-1468 (1993): Manning. D. L. et al., European J. Cancer 30A(5):675-678 (1994); Manning. D. L. et al. Acta Oncologica 34 (5):641-646 (1995); Manning, D. L. et al., U.S. Pat. No. 5,693,465). Expression of pLIV-1, but not pS2, is associated with metastasis of breast cancer cells to regional lymph nodes (Manning et al. U.S. Pat. No. 5,692,465).

In addition, the pathogenesis of various human malignancies, including breast cancer, is affected by proto-oncogenes that encode growth factors and growth factor receptors. Human ErbB2 gene (erbB2, also known as her2, or c-erbB-2), which encodes a 185-kd transmembrane glycoprotein receptor (ErbB2, also known as HER2 or p185.sup.HER2) related to the epidermal growth factor receptor (EGFR), is overexpressed in about 25% to 30% of human breast cancer (Slamon et al., Science 235:177-182 [1987]: Slamon et al. Science 244:707-712 [1989]).

Several lines of evidence support a direct role for ErbB2 in the pathogenesis and clinical aggressiveness of ErbB2-overexpressing tumors. The introduction of ErbB2 into non-neoplastic cells causes their malignant transformation (Hudziak et al. Proc. Natl. Acad. Sci. USA 84:7159-7163 [1987]; DiFiore et al., Science 237:78-182 [1987]). Transgenic mice that express ErbB2 develop mammary tumors (Guy et al., Proc. Natl. Acad. Sci. USA 89:10578-10582 [1992]). ErbB2 overexpression is commonly regarded as a predictor of a poor prognosis in humans, especially in patients with primary disease that involves axillary lymph nodes (Slamon et al. [1987] and [1989], supra: Ravdin and Chamness, Gene 159:19-27 [1995]; and Hynes and Stern, Biochim Biophys Acta 1198:165-184 [1994]).

Antibodies directed against human erbB2 protein products (anti-ErbB2 antibodies) and against proteins encoded by the rat equivalent of the erbB2 gene (neu) (anti-neu protein antibodies) down-modulate cell surface expression of p185 on B104-1-1 cells (NIH-3T3 cells transfected with the neu proto-oncogene) and inhibit colony formation of these cells, Drebin et al., Cell 41:695-706 (1985). Biological effects of anti-neu protein antibodies are reviewed in Myers et al., Meth. Enzym. 198:277-290 (1991). See also WO94/22478 published Oct. 13, 1994.

The anti-ErbB2 antibody, 4D5, exhibited anti proliferative effects on the SKDR3 human breast tumor cell line, inhibiting cellular proliferation by approximately 56%, and sensitizing p185.sup.erbB2 -overexpressing breast tumor cell lines to the cytotoxic effects of TNF-.alpha.. See Hudziak et al., Mol. Cell. Biol. 9(3):1165-1172(1989). See also WO89/06692 published Jul. 27, 1989. The anti-ErbB2 antibodies discussed in Hudziak et al. are further characterized in Fendly et al. Cancer Research 50:1550-1558 (1990); Kotts et al. In Vitro 26(3):59A (1990): Sarup et al. Growth Regulation 1:72-82 (1991): Shepard et al. J. Clin. Immunol. 11(3): 117-127 (1991): Kumar et al. Mol. Cell. Biol. 11(2):979-986 (1991); Lewis et al. Cancer Immunol. Immunother. 37:255-263 (1993); Pietras et al. Oncogene 9:1829-1838 (1994); Vitetta et al. Cancer Research 54:5301-5309 (1994); Sliwkowski et al. J. Biol. Chem. 269(20):14661-14665 (1994): Scott et al. J. Biol. Chem. 266:14300-5 (1991); and D'souza et al. Proc. Natl. Acad. Sci. 91:7202-7206 (1994).

ErbB2 overexpression is also linked to sensitivity and/or resistance to hormone therapy and chemotherapeutic regimens, including CMF (cyclophosphamide, methotrexate, and fluoruracil) and anthracyclines (Baselga et al., Oncology 11(3 Suppl 1):43-48 [1997]). Despite the association of ErbB2 overexpression with poor prognosis, the odds of HER2-positive patients responding clinically to treatment with taxanes were greater than three times those of HER2-negative patients (Ibid), rhuMab HER2 was shown to enhance the activity of paclitaxel (TAXOL.RTM.) and doxorubicin against breast cancer xenografts in nude mice injected with BT-474 human breast adenocarcinoma cells, which express high levels of HER2 (Baselga et al. Breast Cancer, Proceedings of ASCO, Vol. 13. Abstract 53 [1994]).

Because breast and other cancers pose constant threats to health, there is a continuing need to develop treatments for cancers by using methods that target cancer cells without simultaneously harming large numbers of non-cancerous cells, thereby limiting adverse side effects associated with traditional cancer chemotherapy.

SUMMARY OF THE INVENTION

The present invention relates to the discovery of a unique protein. LIV-1-164647, that is overexpressed in some tumor tissues, such as in prostate, colon, lung, breast, and a population of breast tumors that overexpress LIV-1-164647, but do not overexpress ErbB2. The present invention further relates to nucleic acid sequences and amino acid sequences having homology to herein disclosed LIV-1 gene sequence (designated DNA 164647) and the amino acid sequence of LIV-1 protein encoded by DNA 164647. Applicants' discovery that LIV-1-164647 is overexpressed in tumor cells led to the additional discoveries of compositions for detection and treatment of tumor cells and methods of carrying out such detection and treatment.

In one aspect, the present invention relates to a nucleic acid sequence having homology to the nucleic acid sequence of DNA 164647 (SEQ ID NO:3 (coding strand)), or a portion thereof. Preferably the homology is at least approximately 80% homology, more preferably at least approximately 90%, still more preferably at least approximately 95%, and most preferably at least approximately 97% homology. Preferably, the nucleic acid of the invention encodes an aqueous soluble extracellular domain (ECD) that is at least 80% homologous to the DNA 164647 (SEQ ID NO:3) from approximately nucleic acid 73 to approximately 1060. Preferably, the homologous nucleic acid of the invention hybridizes under stringent conditions to a 30 nucleic acid or longer portion of the nucleic acid sequence of DNA 164647 (SEQ ID NO:3) or its complementary sequence, preferably hybridizing under stringent conditions to a 30 nucleotide regions from nucleotide 440 to and including nucleotide 470 of SEQ ID NO:3, or its complementary sequence. In a related embodiment, the homologous nucleic acid of the invention comprises a nucleic acid sequence comprising a sequence that is at least 50%, preferably at least 80%, more preferably at least 90% homologous to the sequence from nucleotide 446 to and including nucleotide 463 of SEQ ID NO:3, or a sequence from nucleotide 2297 to and including 2337 of SEQ ID NO:3, or both sequences. Most preferably, the isolated nucleic acid comprises a sequence from nucleotide 446 to and including nucleotide 464 and/or from nucleotide 2297 to and including 2337. According to the presently disclosed invention, the isolated nucleic acid of the invention comprises a sequence having at least 65%, preferably at least 75%, more preferably at least 85%, still more preferably at least 90%, and most preferably at least 96% homologous to a sequence from approximately nucleotide 412 to and including nucleotide 477 of SEQ ID NO:3, or its complementary sequence. Preferably, the sequence encodes a histidine-rich region of an antigenic polypeptide, preferably an ECD.

In another aspect, the present invention relates to an isolated polypeptide comprising an amino acid sequence having homology to the amino acid sequence (SEQ ID NO:4), or a fragment thereof, encoded by or within DNA 164647, designated herein as LIV-1-164647. Preferably the homology is at least approximately 80% homology, more preferably at least approximately 90%, still more preferably at least approximately 95%, and most preferably at least approximately 97% homology. Preferably, a LIV-1-164647 amino acid sequence of the invention is an aqueous soluble ECD homologous to amino acid 1 to approximately amino acid 327 or a fragment thereof comprising at least 10 amino acids. The region of the ECD is readily determined from a standard hydropathy plot indicating the relatively more hydrophilic region N-terminal of a hydrophobic transmembrane region. In a related embodiment, the homologous amino acid sequence of the invention comprises a sequence from amino acid 126 to and including amino acid 132 of SEQ ID NO:4 (specifically, the amino acid sequence HDHHSHH (SEQ ID NO:17)), or a sequence from amino acid 743 to and including amino acid 755 of SEQ ID NO:4 (specifically, the amino acid sequence SIFEHKIVFRINF (SEQ ID NO:18), or both sequences. The present invention further includes an isolated polypeptide comprising an amino acid sequence having at least 50%, preferably at least 80%, more preferably at least 90% homologous to SEQ ID NO:17. The present invention still further includes an isolated polypeptide comprising an amino acid sequence having at least 20%, more preferably at least 50%, still more preferably at least 80%, and most preferably at least 90% homology to SEQ ID NO:18. In still another embodiment, the invention includes an isolated nucleic acid of SEQ ID NO:3 and an isolated polypeptide of SEQ ID NO:4. The present invention further includes an isolated polypeptide comprising an amino acid sequence having at least 65%, preferably at least 75%, more preferably at least 85%, still more preferably at least 90%, and most preferably at least 96% to a sequence from amino acid 114 to and including amino acid 135 of SEQ ID NO:4. The amino acid sequence from amino acid 114 to 135 is designated SEQ ID NO:19. A still further embodiment includes an isolated polypeptide comprising SEQ ID NO:17 and/or SEQ ID NO:18.

In still another embodiment, the invention includes an isolated polypeptide comprising an amino acid sequence wherein the sequence is at least 98% homologous to the sequence from amino acid 1 to and including amino acid 327 of SEQ ID NO:4, more preferably comprising the ECD of LIV-1-164647. Most preferably, the sequence comprises SEQ ID NO:17, forms a portion of an extracellular domain (ECD), preferably the ECD of LIV-1-164647. The term "portion" as used herein refers to a sequence that comprises at least 7 amino acids of the ECD of LIV-1-164647 from amino acid 1 to and including amino acid 327 of SEQ ID NO:4.

In another embodiment, the present invention concerns an antibody which specifically binds a LIV-1 polypeptide. Preferably, the antibody is a monoclonal antibody. More preferably, the antibody is a human antibody or a humanized antibody. In one embodiment, the antibody reduces activity of overexpressed LIV-1 polypeptide in a cell. In another aspect, the antibody is a monoclonal antibody, which preferably has nonhuman complementarity determining region (CDR) residues and human framework region (FR) residues. The antibody may be labeled and may be immobilized on a solid support. In a further aspect, the antibody is an antibody fragment, a single-chain antibody, or an anti-idiotypic antibody. Preferably, a LIV-1-binding antibody of the invention binds specifically to a polypeptide having at least approximately 80% homology, more preferably at least approximately 90% homology, still more preferably at least approximately 95% homology, and most preferably at least approximately 97% homology to the LIV-1 ECD nucleic acid sequence, or a fragment thereof, encoded within the ECD coding region (nucleotides 1-1000) of DNA 164647 (SEQ ID NO:3). More preferably, a LIV-1-binding antibody of the invention binds specifically to a polypeptide having at least 80% homology, more preferably at least approximately 90% homology, still more preferably at least approximately 95% homology, and most preferably at least approximately 97% homology to the amino acid sequence of LIV-1 ECD (amino acids 1-327 of SEQ ID NO:4). In a preferred embodiment, the present invention concerns an isolated antibody which specifically binds a LIV-1 polypeptide encoded by a nucleic acid sequence comprising a nucleic acid sequence having at least 65%, preferably at least 75%, more preferably at least 85%, still more preferably at least 90%, and most preferably at least 96%, homology to a sequence from nucleotide 446 to and including nucleotide 463 of SEQ ID NO:3, or the nucleic acid sequence from 2297 to and including 2337 of SEQ ID NO:3, or both nucleic acid sequences. In another preferred embodiment, the present invention concerns an isolated antibody which specifically binds a LIV-1 polypeptide comprising the amino acid sequence having at least 65%, preferably at least 75%, more preferably at least 85%, still more preferably at least 90%, and most preferably at least 96% homology to a sequence from amino acid 126 to and including amino acid 132 of SEQ ID NO:4, or the amino acid sequence from amino acid 743 to and including amino acid 755 of SEQ ID NO:4, or both amino acid sequences.

In still another embodiment, the invention concerns an antibody, preferably a monoclonal antibody, that specifically binds the same epitope of LIV-1, preferably LIV-1-1164647, that is bound by any one of the monoclonal antibodies produced by the hybridoma cell lines deposited with the American Type Culture Collection (ATCC) as disclosed herein.

In a further embodiment, the invention includes an antibody that binds to a polypeptide comprising a sequence from amino acid 1 to and including amino acid 147 of SEQ ID NO:4. In another embodiment, the antibody binds a polypeptide comprising amino acid 148 to and including amino acid 298 of SEQ ID NO:4. Preferably, the antibodies are monoclonal antibodies. More preferably, the monoclonal antibodies are human antibodies or humanized antibodies.

In another aspect, the invention concerns a composition comprising an antibody which binds LIV-1 polypeptide in an admixture with a pharmaceutically acceptable carrier. In one aspect, the composition comprises a therapeutically effective amount of the antibody. In another aspect, the composition comprises a further active ingredient, which may, for example, be a further antibody or a cytotoxic or chemotherapeutic agent. Preferably, the composition is sterile.

In a further embodiment, the invention concerns a nucleic acid encoding an anti-LIV-1 antibody according to the invention, and vectors and recombinant host cells comprising such nucleic acid.

In a still further embodiment, the invention concerns a method for producing an anti-LIV-1 antibody by culturing a host cell transformed with nucleic acid encoding the antibody under conditions such that the antibody is expressed, and recovering the antibody from the cell culture.

The invention further concerns antagonists and agonists of a LIV-1 polypeptide, which antagonists inhibit one or more of the functions or activities of the LIV-1 polypeptide and which agonists mimic one or more of the functions or activities of the LIV-1 polypeptide. Preferably the LIV-1 polypeptide is the LIV-1-164647 polypeptide whose functions or activities are antagonized or agonized.

In another embodiment, the invention concerns a method for determining the presence of a LIV-1 polypeptide or fragment thereof comprising exposing a cell suspected of containing the LIV-1 polypeptide to an anti-LIV-1 antibody of the invention and determining binding of the antibody to the cell.

In yet another embodiment, the present invention concerns a method of diagnosing tumor in a mammal, comprising detecting the level of expression of a gene encoding a LIV-1 polypeptide in a test sample of tissue cells obtained from the mammal, and in a control sample of known normal tissue cells of the same cell type, wherein a higher expression level in the test sample indicates the presence of tumor in the mammal from which the test tissue cells were obtained.

In another embodiment, the present invention concerns a method of diagnosing tumor in a mammal, comprising contacting an anti-LIV-1 antibody with a test sample of tissue cells obtained from the mammal, and detecting the formation of a complex between the anti-LIV-1 antibody and the LIV-1 polypeptide in the test sample. The detection may be qualitative or quantitative, and may be performed in comparison with monitoring the complex formation in a control sample of known normal tissue cells of the same cell type. A larger quantity of complexes formed in the test sample indicates the presence of tumor in the mammal from which the test tissue cells were obtained. The antibody preferably carries a detectable label. Complex formation can be monitored, for example, by light microscopy, flow cytometry, fluorimetry, or other techniques known in the art.

For the methods of diagnosing, the test sample is usually obtained from an individual suspected to have neoplastic cell growth or proliferation (e.g. cancerous cells).

In another embodiment, the invention involves a method of diagnosing breast tumor tissue as tissue that overexpresses LIV-1 protein and expresses normal levels of ErbB2. The method comprises providing a test sample of tissue suspected of being cancerous, contacting the test sample with an antibody to the naturally occurring form of the LIV-1 gene product, contacting the same or duplicate test sample with an anti-ErbB2 antibody, detecting the relative binding of the antibodies to the test sample compared to a control sample, where the control may be a positive control, a negative control, or both. A test sample that overexpresses LIV-1 gene product (relative to normal tissue), but does not overexpress ErbB2 protein (relative to normal tissue), is diagnosed as a member of the population of breast tumors to be treated by the compositions and methods of the invention. Useful in the diagnostic assay method of the invention are anti-ErbB2 antibodies that bind the extracellular domain of the ErbB2 receptor, and preferably bind to the epitope 4D5 or 3H4 within the ErbB2 extracellular domain sequence. Mole preferably, the antibody is the antibody 4D5. Other preferred ErbB2-binding antibodies include, but are not limited to, antibodies 7C2, 7F3, and 2C4. Information regarding anti-ErbB2 antibodies is found, for example, in Hudziak, R. M. et al. U.S. Pat. No. 5,772,997, incorporated herein by reference in its entirety.

In another aspect, the present invention concerns a cancer diagnostic kit, comprising an anti-LIV-1-164647 antibody and a carrier (e.g. a buffer) in suitable packaging. The kit preferably contains instructions for using the antibody to detect the LIV-1 polypeptide.

In yet another aspect, the invention concerns a method for inhibiting the growth of tumor cells comprising exposing a cell which overexpresses a LIV-1 polypeptide to an effective amount of an agent inhibiting the expression and/or activity of the LIV-1 polypeptide. The agent preferably is an anti-LIV-1-164647 antibody, a small organic and inorganic molecule, peptide, phosphopeptide, antisense or ribozyme molecule, or a triple helix molecule. In a specific aspect, the agent, e.g. anti-LIV-1-164647 antibody induces cell death, or at least slows cell growth sufficiently to allow other methods of cancer treatment to be administered. In a further aspect, the tumor cells are further exposed to radiation treatment and/or a cytotoxic or chemotherapeutic agent.

In yet another aspect, the invention concerns a method for the treatment of a human patient susceptible to or diagnosed with a disorder characterized by overexpression of LIV-1 gene product without overexpression of ErbB2 receptor. In an embodiment, the method comprises administering a therapeutically effective amount of an anti-LIV-1 polypeptide antibody, where administration may be intravenous, subcutaneous, or other pharmaceutically acceptable method of antibody delivery. Preferably the antibody specifically binds the naturally occurring form of the LIV-1-164647 polypeptide, wherein the binding is preferably to the extracellular domain or a fragment thereof. Preferably, the initial dose (or doses) as well as the subsequent maintenance dose or doses are administered subcutaneously. Optionally, where the patient's tolerance of the anti-LIV-1 antibody is unknown, the initial dose is administered by intravenous infusion, followed by subcutaneous administration of the maintenance doses it the patient's tolerance for the antibody is acceptable. According to the embodiment of the invention, the initial dose or doses is followed by subsequent doses of equal or smaller amounts of antibody at intervals sufficiently close to maintain the trough serum concentration of antibody at or above an efficacious target level. Preferably, an initial dose or individual subsequent dose does not exceed 100 mg/kg, and each subsequent dose is at least 1 .mu.g/kg. The choice of delivery method for the initial and maintenance doses is made according to the ability of the animal or human patient to tolerate introduction of the antibody into the body. Where the antibody is well-tolerated, the time of infusion may be reduced. The choice of delivery method as disclosed for this embodiment applies to all drug delivery regimens contemplated according to the invention.

In a further aspect, the invention provides a method of treating LIV-1 gene product-overexpressing cancer (lacking overexpression of ErbB2) in a human patient comprising administering to the patient effective amounts of an anti-LIV-1 antibody (which antibody preferably binds the extracellular domain of LIV-1 gene product) and a chemotherapeutic agent. In one embodiment of the invention, the chemotherapeutic agent in a toxoid including, but not limited to, paclitaxel and doxetaxel. In another embodiment, the chemotherapeutic agent is an anthracyline derivative including, but not limited to, doxorubicin and epirubicin. In still another embodiment, the chemotherapeutic agent is not administered to the patient simultaneously with the anti-LIV-1 antibody. One or more additional chemotherapeutic agents may also be administered to the patient.

The disorder to be treated by a method of the invention preferably is a benign or malignant tumor characterized by the overexpression of the LIV-1 gene product. Preferably, the malignant cells of the tumor express approximately the same level of ErbB2 (or less) as a non-cancerous cell of the same type. For example, the disorder to be treated is a cancer, such as breast cancer, lung cancer, and prostate cancer.

Accordingly, one aspect of the invention involves compounds that bind to the LIV-1 protein and inhibit its activity. Preferably the compounds bind to the extracellular region of the LIV-1 protein and inhibit its activity. In an embodiment of the invention, the inhibiting compounds are antibodies specific to the LIV-1 gene product or fragments thereof. Preferably, the inhibiting compounds of the invention bind specifically to the extracellular region of the LIV-1 protein.

In another aspect, the invention involves compounds that block the binding of an activating ligand of LIV-1 protein. Such ligand-blocking compounds include, but are not limited to polypeptides, proteins, antibodies and the like. Preferably the ligand-blocking compounds specifically block the activity of a LIV-1 activating ligand. More preferably, the ligand-blocking compounds of the invention inhibit growth of a LIV-1-expressing cell.

In another aspect, the invention involves a method for identifying a compound capable of inhibiting the expression and/or activity of a LIV-1 polypeptide, comprising contacting a candidate compound with a LIV-1 polypeptide under conditions and for a time sufficient to allow these two components to interact. In a specific aspect, either the candidate compound or the LIV-1 polypeptide is immobilized on a solid support. In another aspect, the non-immobilized component carries a detectable label.

In yet another aspect, the invention concerns an article of manufacture, comprising a container; a composition within the container comprising an anti-LIV-1 antibody that binds the LIV-1 protein (preferably binding to the extracellular domain or a fragment thereof) or binds an activating ligand of the LIV-1 protein; and optionally a label on or associated with the container that indicates that the composition can be used for treating a condition characterized by overexpression of LIV-1 without overexpression of ErbB2. According to another embodiment of the invention, the article of manufacture further includes a package insert comprising instructions to administer the anti-LIV-1 antibody subcutaneously for at least one of the doses, preferably for all of the subsequent doses following the initial dose, most preferably for all doses.

Where the methods and compositions of the invention comprise an anti-LIV-1 antibody, which specifically and preferably binds the extracellular domain of a LIV-1 gene product, or a fragment of the extracellular domain. The compositions of the invention preferably include a humanized LIV-1 antibody. Thus, the invention further pertains to a composition comprising an antibody that specifically and preferably binds the extracellular domain of LIV-1 gene product, and pertains to the use of the antibody for treating LIV-1+/ErbB2-expressing cancer in a human, e.g., LIV-1 overexpressing cancer that does not coexpress high levels of ErbB2. Preferably the antibody is a monoclonal antibody, e.g., humanized anti-LIV-1 monoclonal antibody that binds to the extracellular domain (or a portion of the extracellular domain) of LIV-1 (hereinafter anti-LIV-1) The antibody may be an intact antibody (e.g., an intact IgG.sub.1 antibody) or an antibody fragment (e.g., a Fab, F(Ab).sub.2, diabody, and the like). The variable light chain and variable heavy chain regions of humanized anti-LIV-1 antibody.

These and other advantages and features of the present invention will become apparent to those persons skilled in the art upon reading the details of the invention as more fully set forth below and in the appended claims.

BRIEF DESCRIPTION OF THE DRAWINGS

FIGS. 1A-1C are the nucleic acid sequence (SEQ ID NO:1 (coding sequence). FIGS. 1A-1 to 1A-2) and the amino acid sequence (SEQ ID NO:2, FIG. 1B) of the LIV-1 protein. The dashed overlined portion is predicted to be a signal sequence (approximately amino acids 1 to 20). The predicted extracellular domain of LIV-1 protein is that portion of the LIV-1 amino acid sequence underscored by a dashed line (approximately amino acids 24 to 312). The predicted transmembrane domain extends from approximately amino acid 318 to approximately amino acid 367. The approximate positions of the domains were predicted using a standard hydropathy analysis program. A nucleic acid sequence (SEQ ID NO:5) encoding a portion of LIV-1 and useful in microarray analysis is shown in FIG. 1C.

FIGS. 2A-2B are the nucleic acid sequence and amino acid sequence, respectively, corresponding to DNA 164647. FIGS. 2A1-2A5 is the nucleotide sequence of DNA 164647 that is a cDNA encoding a native sequence LIV-1 protein. SEQ ID NO:3 is the coding strand of DNA 164647. FIG. 2B is the derived amino acid sequence (SEQ ID NO:4) of a native LIV-1 polypeptide encoded by DNA 164647.

FIGS. 3A-1-3A-9 is an alignment of SEQ ID NO:1 and SEQ ID NO:3 nucleic acid sequences.

FIGS. 4-1-4-3 is an alignment of SEQ ID NO:2 and SEQ ID NO:4 amino acid sequences. The sequences differ in the ECD (near amino acid 130 of SEQ ID NO:4) and C-terminal region beyond about amino acid 740 of SEQ ID NO:4. A single amino acid difference was found at amino acid 651 of SEQ ID NO:4.

FIG. 5 is a flow chart illustrating the FLIP cloning method up to the restriction digestion selection step, as described herein. The shaded boxes flanking the vector sequence represent the target gene sequences.

FIG. 6 is a graphical representation of a fluorescent activated cell sorting (FACS) analysis in which an anti-LIV-1-164647 monoclonal antibody was shown to bind primarily to the surface of 3T3 cells transfected with DNA 164647. The term "pRK5" refers cells transfected with vector lacking a LIV-1-164647 insert. The term "pRK5-LIV-1-164647" refers to cells transfected with vector expressing full length LIV-1-164647.

FIG. 7 is a bar graph demonstrating that the LIV-1-164647 extracellular domain is expressed on the surface of cells transfected with DNA encoding the full-length LIV-1-164647 protein.

DESCRIPTION OF THE EMBODIMENTS

1. Definitions

As used herein, the term "LIV-1" refers to a gene or its encoded protein, which gene transcript is detected in above normal levels in some cancer cells. More specifically, a LIV-1 gene or protein of the present invention is one which is encoded by DNA 164647 (SEQ ID NO:3) and has the deduced amino acid sequence of SEQ ID NO:4. As used herein, the term LIV-1 refers to LIV-1-164647 where the disclosure refers to a nucleic acid comprising at least 21 nucleotides of SEQ ID NO:3, or where the disclosure refers to an amino acid sequence comprising at least 7 amino acids of SEQ ID NO:4 as disclosed herein. According to the invention. LIV-1-164647 is expressed in higher than normal amounts in a cell, while the gene encoding ErbB2 receptor is not expressed in higher than normal amounts. Such higher than normal expression is termed "overexpression" of a gene or protein. The term "LIV-1" or "LIV-1-164647" may be used to refer to a LIV-1 gene or its encoded protein. Generally, where a protein or peptide is contemplated, the term "LIV-1 protein" will be used.

The term "LIV-1 gene product" or "LIV-1 protein" refers to the expressed protein product of the gene, preferably a polypeptide or protein form of the gene product. According to the invention, a polypeptide or protein form of the LIV-1 gene product includes a soluble form of the gene product (i.e. the extracellular domain (ECD) of the LIV-1 gone product), which soluble form is useful as an antigen for raising anti-LIV-1 gene product antibodies that bind the extracellular domain of full length LIV-1 gene product and inhibit its activation. It is understood that LIV-1 gene product may also refer to the messenger RNA (mRNA) gene product and, where appropriate, the distinction between protein and mRNA is made. A LIV-1 protein according to the invention is encoded by a nucleic acid of the invention comprising a sequence at least 80% homologous to the DNA 164647 (SEQ ID NO:3 or its complement; FIG. 2A), preferably at least approximately 90% homologous, more preferably at least approximately 95%, and most preferably at least approximately 97% homologous to SEQ ID NO:3 or its complement), or a portion thereof. A LIV-1 nucleic acid of the invention hybridizes under stringent conditions to SEQ ID NO:3 or its complement) or a portion thereof. A LIV-1 protein of the invention is at least 80% homologous to the amino acid sequence encoded by DNA 164647 (LIV-1 polypeptide SEQ ID NO:4; FIG. 2B), preferably at least approximately 90% homologous, more preferably at least approximately 95%, and most preferably at least approximately 97% homologous to SEQ ID NO:4, or a fragment thereof.

The terms "anti-LIV-1 antibody," "LIV-1 antibody," and grammatically analogous terms refer to an antibody which binds specifically to at least a portion of the extracellular domain of the LIV-1-164647 protein having a predicted amino acid sequence of SEQ ID NO:4 (the predicted full length amino acid sequence of LIV-1-164647 gene). Preferably, the antibody binds to the extracellular domain of LIV-1 gene product, more preferably binding to the same epitope as epitopes A, B, or C to which the monoclonal antibodies disclosed herein bind. Even more preferably, the anti-LIV-1-164647 antibody binds to a polypeptide having at least 65% homology to a sequence from amino acid 114 to and including amino acid 135 of SEQ ID NO:4. Preferably, an anti-LIV-1 antibody of the invention is human or humanized when the antibody is to be used to treat a human patient.

The antibody of the invention is preferably one which binds specifically to human LIV-1-164647, meaning that it does not significantly cross-react with other proteins. In such embodiments, the extent of binding of the antibody to proteins other than LIV-1 gene product will be less than about 10% as determined by fluorescence activated cell sorting (FACS) analysis or radioimmunoprecipitation (RIA).

The term "antibody" is used in the broadest sense and specifically covers, for example, single anti-LIV-1 monoclonal antibodies (including agonist, antagonist, and neutralizing antibodies), anti-LIV-1 antibody compositions with polyepitopic specificity, single chain anti-LIV-1 antibodies. The term "monoclonal antibody" as used herein refers to an antibody obtained from a population of substantially homogeneous antibodies, i.e., the individual antibodies comprising the population are identical except for possible naturally-occurring mutations that may be present in minor amounts.

"Antibodies" (Abs) and "immunoglobulins" (Igs) are glycoproteins having the same structural characteristics. While antibodies exhibit binding specificity to a specific antigen, immunoglobulins include both antibodies and other antibody-like molecules which lack antigen specificity. Polypeptides of the latter kiln are, for example, produced at low levels by the lymph system and at increased levels by myelomas. The term "antibody" is used in the broadest sense and specifically covers, without limitation, intact monoclonal antibodies, polyclonal antibodies, multispecific antibodies (e.g. bispecific antibodies) formed from at least two intact antibodies, and antibody fragments so long as they exhibit the desired biological activity.

"Native antibodies" and "native immunoglobulins" are usually heterotetrameric glycoproteins of about 150,000 daltons composed of two identical light (L) chains and two identical heavy (H) chains. Each light chain is linked to a heavy chain by one covalent disulfide bond, while the number of disulfide linkages varies among the heavy chains of different immunoglobulin isotypes. Each heavy and light chain also has regularly spaced intrachain disulfide bridges. Each heavy chain has at one end a variable domain (V.sub.H) followed by a number of constant domains. Each light chain has a variable domain at one end (V.sub.L) and a constant domain at its other end; the constant domain of the light chain is aliened with the first constant domain of the heavy chain, and the light-chain variable domain is aligned with the variable domain of the heavy chain. Particular amino acid residues are believed to form an interface between the light- and heavy-chain variable domains.

The term "variable" refers to the fact that certain portions of the variable domains differ extensively in sequence among antibodies and are used in the binding and specificity of each particular antibody for its particular antigen. However, the variability is not evenly distributed throughout the variable domains of antibodies. It is concentrated in three segments called complementarity-determining regions (CDRs) or hypervariable regions both in the light-chain and the heavy-chain variable domains. The more highly conserved portions of variable domains are called the framework (FR). The variable domains of native heavy and light chains each comprise four FR regions, largely adopting a -sheet configuration, connected by three CDRs, which form loops connecting, and in some cases forming part of, the -sheet structure. The CDRs in each chain are held together in close proximity by the FR regions and, with the CDRs from the other chain, contribute to the formation of the antigen-binding site of antibodies (see Kabat et al. NIH Publ. No.91-3242, Vol. 1 pages 647-669 (1991)). The constant domains are not involved directly in binding an antibody to an antigen, but exhibit various effector functions, such as participation of the antibody in antibody-dependent cellular toxicity.

The term "hypervariable region" when used herein refers to the amino acid residues of an antibody which are responsible for antigen-binding. The hypervariable region comprises amino acid residues from a "complementarity determining region" to "CDR" (i.e., residues in the light chain variable domain and residues in the heavy chain variable domain; Kabat et al., Sequences of Proteins of Immunological Interest, 5th Ed. Public Health Service, National Institute of Health, Bethesda, Md. [1991]) and/or those residues from a "hypervariable loop" (i.e., residues in the light chain variable domain and residues in the heavy chain variable domain; Clothia and specificity, the monoclonal antibodies are advantageous in that they are synthesized by the hybridoma culture, uncontaminated by other immunoglobulins. The modifier "monoclonal" indicates the character of the antibody as being obtained from a substantially homogeneous population of antibodies, and is not to be construed as requiring production of the antibody by any particular method. For example, the monoclonal antibodies to be used in accordance with the present invention may be made by the hybridoma method first described by Kohler et al., Nature, 256:495 [1975], or may be made by recombinant DNA methods (see, e.g. U.S. Pat. No. 4,816,567). The monoclonal antibodies may also be isolated from phage antibody libraries using the techniques described in Clackson et al., Nature, 352:624-628 [1991] and Marks et al., J. Mol. Biol. 222:581-597 (1991), for example.

The monoclonal antibodies herein specifically include "chimeric" antibodies in which a portion of the heavy and/or light chain is identical with or homologous to corresponding sequences in antibodies derived from a particular species or belonging to a particular antibody class or subclass, while the remainder of the chain(s) is identical with or homologous to corresponding sequences in antibodies derived from another species or belonging to another antibody class or subclass, as well as fragments of such antibodies, so long as they exhibit the desired biological activity (U.S. Pat. No. 4,816,567; Morrison et al., Proc. Natl. Acad. Sci. USA. 81:6851-6855 [1984]). Chimeric antibodies of interest herein include human constant region sequences together with antigen bindings regions of rodent (e.g. murine) origin, or "primatized" antibodies comprising variable domain antigen-binding sequences derived from a non-human primate (e.g. Old World Monkey, Ape, macaque, etc.), or antigen binding regions derived from antibodies generated in other non-human species that have been immunized with the antigen of interest.

"Humanized" forms of non-human (e.g., rodent) antibodies are chimeric immunoglobulins, immunoglobulin chains or fragments thereof (such as Fv, Fab, Fab', F(ab').sub.2 or other antigen-binding subsequences of antibodies) which contain minimal sequence derived from non-human immunoglobulin. For the most part, humanized antibodies are human immunoglobulins (recipient antibody) in which residues from a hypervariable region of the recipient are replaced by residues from a hypervariable region of a non-human species (donor antibody) such as mouse, rat or rabbit having the desired specificity, affinity, and capacity. In some instances, framework region (FR) residues of the human immunoglobulin are replaced by corresponding non-human residues. Furthermore, humanized antibodies may comprise residues which are found neither in the recipient antibody nor in the donor antibody. These modifications are made to further refine and maximize antibody performance. In general, the humanized antibody will comprise substantially all of at least one, and typically two, variable domains, in which all or substantially all of the hypervariable loops correspond to those of a non-human immunoglobulin and all or substantially all of the FRs are those of a human immunoglobulin sequence. The humanized antibody optionally also will comprise at least a portion of an immunoglobulin constant region (Fc), typically that of a human immunoglobulin. For further details, see, Jones et al., Nature, 311:522-525 (1986); Reichmann et al., Nature, 332:323-329 [1988]; and Presta, Curr. Op. Struct. Biol. 2:593-596 (1992).

"Single-chain Fv" or "sFv" antibody fragments comprise the V.sub.H and V.sub.L domains of antibody, wherein these domains are present in a single polypeptide chain. Preferably, the Fv polypeptide further comprises a polypeptide linker between the V.sub.H and V.sub.L domains which enables the sFv to form the desired structure for antigen binding. For a review of sFv see Pluckthun in The Pharmacology of Monoclonal Antibodies, vol. 113, Rosenhurg and Moore eds., Springer-Verlag, New York, pp. 269-315 (1994).

The term "diabodies" refers to small antibody fragments with two antigen-binding sites, which fragments comprise a heavy-chain variable domain (V.sub.H) connected to a light-chain variable domain (V.sub.L) in the same polypeptide chain (V.sub.H-V.sub.L). By using a linker that is too short to allow pairing between the two domains on the same chain, the domains are forced to pair with the complementary domains of another chain and create two antigen-binding sites. Diabodies are described more fully in, for example, EP 404,097; WO 93/11161; and Hollinger et al., Proc. Natl. Acad. Sci. USA. 90:6444-6448 (1993).

An "isolated" antibody is one which has been identified and separated and/or recovered from a component of its natural environment. Contaminant components of its natural environment are materials which would interfere with diagnostic or therapeutic uses for the antibody, and may include enzymes, hormones, and other proteinaceous or nonproteinaceous solutes. In preferred embodiments, the antibody will be purified (1) to greater than 95% (by weight of antibody as determined by the Lowry method, and most preferably more than 99% by weight, (2) to a degree sufficient to obtain at least 15 residues of N-terminal or internal amino acid sequence by use of a spinning cup sequenator, or (3) to homogeneity by SDS-PAGE under reducing or nonreducing conditions using Coomassie blue or, preferably, silver stain. Isolated antibody includes the antibody in situ within recombinant cells since at least one component of the antihody's natural environment will not be present. Ordinarily, however, isolated antibody will be prepared by at least one purification step.

The term "overexpression," as used herein refers to overexpression of a gene and/or its encoded protein in a cell, such as a cancer cell. A cancer cell that "overexpresses" a protein is one that has significantly higher levels of that protein compared to a noncancerous cell of the same tissue type. For example, according to the present invention, the overexpression of a protein LIV-1 protein may be caused by gene amplification or by increased transcription or translation.

Overexpression of a LIV-1 protein may be determined in a diagnostic or prognostic assay by evaluating increased levels of a LIV-1 mRNA in a cell or tissue (e.g. via a quantitative PCR method) or by detecting a LIV-1 protein present on the surface of a cell (e.g. via an immunohistochemistry assay). Alternatively, or additionally, one may measure levels of LIV-1-encoding nucleic acid in the cell, e.g. via fluorescent in situ hybridization (FISH; see WO98/45479 published October, 1998), southern blotting, or polymerase chain reaction (PCR) techniques, such as real time quantitative PCR (RT-PCR). One may also study LIV-1 overexpression by measuring shed antigen (e.g., LIV-1 extracellular domain) in a biological fluid such as serum by contacting the fluid or other sample with an antibody that binds to a LIV-1 protein or fragment thereof. Various in vitro and in vivo assays are available to the skilled practitioner. For example, one may expose a fluid or tissue comprising a LIV-1 protein or fragment thereof, or cells within the body of the patient to an antibody which is optionally labeled with a detectable label, e.g. a radioactive isotope, and binding of the antibody to cells in a sample or the patient can be evaluated for overexpression, e.g. by external scanning for radioactivity or by analyzing a biopsy taken from a patient previously exposed to the antibody.

A cell that "overexpresses" LIV-1 has significantly higher than normal LIV-1 nucleic acid levels compared to a noncancerous cell of the same tissue type. Typically, the cell is a cancer cell, e.g. a breast, ovarian, prostate, stomach, endometrial, salivary gland, lung, kidney, colon, thyroid, pancreatic or bladder cell. The cell may also be a cell line such as SKBR3, BT474, Calu 3, MDA-MB-453, MDA-MB-361 or SKOV3.

Conversely, a cancer that is "not characterized by overexpression of a LIV-1 protein or a LIV-1 gene is one which, in a diagnostic assay, does not express higher than normal levels of LIV-1 gene or LIV-1 protein compared to a noncancerous cell of the same tissue type.

The terms "cancer" and "cancerous" refer to or describe the physiological condition in mammals that is typically characterized by unregulated cell growth. Examples of cancer include but are not limited to, carcinoma, lymphoma, blastoma, sarcoma, and leukemia. More particular examples of such cancers include highest cancer, prostate cancer, colon cancer, squamous cell cancer, small-cell lunge cancer, non-small cell lunar cancer, gastrointestinal cancer, pancreatic cancer, glioblastoma cervical cancer, ovarian cancer, liver cancer, bladder cancer, hepatoma, colorectal cancer, endometrial carcinoma, salivary gland carcinoma kidney cancer, liver cancer, vulval cancer, thyroid cancer, hepatic carcinoma and various types of head and neck cancer.

The phrases "gene amplification" and "gene duplication" are used interchangeably and refer to a process by which multiple copies of a gene or gene fragment are formed in a particular cell or cell line. The duplicated region (a stretch of amplified DNA) is often referred to as "amplicon." Usually, the amount of the messenger RNA (mRNA) produced, i.e., the level of gene expression, also increases in the proportion of the number of copies made of the particular gene expressed.

"Tumor", as used herein, refers to all neoplastic cell growth and proliferation, whether malignant or benign, and all pre-cancerous and cancerous cells and tissues.

"Treatment" is an intervention performed with the intention of preventing the development or altering the pathology of a disorder. Accordingly, "treatment" refers to both therapeutic treatment and prophylactic or preventative measures. Those in need of treatment include those already with the disorder as well as those in which the disorder is to be prevented. In tumor (e.g., cancer) treatment, a therapeutic agent may directly decrease the pathology of tumor cells, or render the tumor cells more susceptible to treatment by other therapeutic agents, e.g., radiation and/or chemotherapy.

The "pathology" of cancer includes all phenomena that compromise the well-being of the patient. This includes, without limitation, abnormal or uncontrollable cell growth, metastasis, interference with the normal functioning of neighboring cells, release of cytokines or other secretory products at abnormal levels, suppression or aggravation of inflammatory or immunological response, etc.

"Mammal" for purposes of treatment refers to any animal classified as a mammal, including humans, domestic and farm animals, and zoo, sports, or pet animals, such as dogs, horses, cats, cattle, pigs, sheep, etc. Preferably, the mammal is human.

"Carriers" as used herein include pharmaceutically acceptable carriers, excipients, or stabilizers which are nontoxic to the cell or mammal being exposed thereto at the dosages and concentrations employed. Often the physiologically acceptable carrier is an aqueous pH buffered solution. Examples of physiologically acceptable carriers include buffers such as phosphate, citrate, and other organic acids, antioxidants including ascorbic acid; low molecular weight (less than about 10 residues) polypeptide; proteins, such as serum albumin, gelatin, or immunoglobulins; hydrophilic polymers such as polyvinylpyrrolidone; amino acids such as glycine, glutamine, asparagine, arginine or lysine; monosaccharides, disaccharides, and other carbohydrates including glucose, mannose, or dextrins; chelating agents such as EDTA; sugar alcohols such as mannitol or sorbitol; salt-forming, counterions such as sodium; and/or nonionic surfactants such as TWEEN.TM., polyethylene glycol (PEG), and PLURONICS.TM..

Administration "in combination with" one or more further therapeutic agents includes simultaneous (concurrent) and consecutive administration in any order.

The term "cytotoxic agent" as used herein refers to a substance that inhibits or prevents the function of cells and/or causes destruction of cells. The term is intended to include radioactive isotopes (e.g., I.sup.131, I.sup.125, Y.sup.90 and Re.sup.186), chemotherapeutic agents, and toxins such as enzymatically active toxins of bacterial, fungal, plant or animal origin, or fragments thereof.

A "chemotherapeutic agent" is a chemical compound useful in the treatment of cancer. Examples of chemotherapeutic agents include adriamycin, doxorubicin, epirubicin, 5-fluorouracil, cytosine arabinoside ("Ara-C"), cyclophosphamide, thiotepa, busulfan, cytoxin, taxoids, e.g., paclitaxel (Taxol, Bristol-Myers Squibb Oncology, Princeton, N.J.), and doxetaxel (Taxotere, Rhone-Poulenc Rorer, Antony, Rnace), toxotere, methotrexate, cisplatin, melphalan, vinblastine, bleomycin, etoposide, ifosfamide, mitomycin C, mitoxantrone, vincristine, vinorelbine, carboplatin, teniposide, daunomycin, carminomycin, aminopterin, dactinomycin, mitomycins, esperamicins (see U.S. Pat. No. 4,675,187), 5-FU, 6-thioguanine, 6-mercaptopurine, actinomycin D, VP-16, chlorambucil, melphalan, and other related nitrogen mustards. Also included in this definition are hormonal agents that act to regulate or inhibit hormone action on tumors such as tamoxifen and onapristone.

A "growth inhibitory agent" when used herein refers to a compound or composition which inhibits growth of a cell, especially cancer cell overexpressing any of the genes identified herein, either in vitro or in vivo. Thus, the growth inhibitory agent is one which significantly reduces the percentage of cells overexpressing such genes in S phase. Examples of growth inhibitory agents include agents that block cell cycle progression (at a place other than S phase), such as agents that induce G1 arrest and M-phase arrest. Classical M-phase blockers include the vincas (vincristine and vinblastine), taxol, and topo II inhibitors such as doxorubicin, epirubicin, daunorubicin, etoposide, and bleomycin. Those agents that arrest GI also spill over into S-phase arrest, for example. DNA alkylating agents such as tamoxifen, prednisone, dacarbazine, mechlorethamine, cisplatin, methotrexate, 5-fluorouracil, and ara-C. Further information can be found in The Molecular Basis of Cancer, Mendelsohn and Israel, eds., Chapter 1, entitled "Cell cycle regulation, oncogens, and antineoplastic drugs" by Murakami et al., (WB Saunders; Philadelphia, 1995), especially p. 13.

"Doxorubicin" is an athracycline antibiotic. The full chemical name of doxorubicin is (85-cis)-10-[(3-amino-2,3,6-trideoxy-.alpha.-L-lyxo-hexopyranosyl)oxy]-7,- 8,9,10-tetrahydro-6,8,11-trihydroxy-8-(hydroxyacetyl)-1-methoxy-5,12-napht- hacenedione.

The term "cytokine" is a generic term for proteins released by one cell population which act on another cell as intercellular mediators. Examples of such cytokines are lymphokines, monokines, and traditional polypeptide hormones. Included among the cytokines are growth hormone such as human growth hormone, N-methionyl human growth hormone, and bovine growth hormone; parathyroid hormone; thyroxine; insulin; proinsulin; relaxin; prorelaxin; glycoprotein hormones such as follicle stimulating hormone (FSH), thyroid stimulating hormone (TSH), and luteinizing hormone (LH); hepatic growth factor; fibroblast growth factor; prolactin; placental lactogen; tumor necrosis factor-.alpha. and -.beta.; mullerian-inhibiting substance; mouse gonadotropin-associatcd peptide; inhibin; activin; vascular endothelial growth factor; integrin; thrombopoietin (TPO); nerve growth factors such as NGF-.beta.; platelet-growth factor; transforming growth factors (TGFs) such as TGF-.alpha. and TGF-.beta.; insulin-like growth factor-I and -II; erythropoietin (EPO); osteoinductive factors; interferons such as interferon-.alpha., -.beta., and -.gamma.; colony stimulating factors (CSFs) such as macrophage-CSF (M-CSF); granulocyte-macrophage-CSF (GM-CSF); and granulocyte-CSF (G-CSF); interleukins (ILs) such as IL-1, IL-1.alpha., IL-2, IL-3, IL-4, IL-5, IL-6, IL-7, IL-8, IL9, IL11, IL12; a tumor necrosis factor such as TNF-.alpha. or TNF-.beta.; and other polypeptide factors including LIF and kit ligand (KL). As used herein, the term cytokine includes proteins from natural sources or from recombinant cell culture and biologically active equivalents of the native sequence cytokines.

The term "prodrug" as used in this application refers to a precursor or derivative form of a pharmaceutically active substance that is less cytotoxic to tumor cells compared to the parent drug and is capable of being enzymatically activated or converted into the more active parent form. See, e.g., Wilman, "Prodrugs in Cancer Chemotherapy" Biochemical Society Transactions, 14, pp. 375-382, 615th Meeting Belfast (1986) and Stella et al., "Prodrugs: A Chemical Approach to Targeted Drug Delivery." Directed Drug Delivery, Borchardt et al., (ed.), pp. 247-267. Humana Press (1985). The prodrugs of this invention include, but are not limited to, phosphate-containing prodrugs, thiophosphate-containing prodrugs, sulfate-containing prodrugs, peptide-containing prodrugs. D-amino acid-modified prodrugs, glycosylated prodrugs, .beta.-lactam-containing prodrugs, optionally substituted phenoxyacetamide-containing prodrugs or optionally substituted phenylacetamide-containing prodrugs. 5-fluorocytosing and other 5-fluorouridine prodrugs which can be converted into the more active cytotoxic free drug. Examples of cytotoxic drugs that can be derivatized into a prodrug form for use in this invention include, but are not limited to, those chemotherapeutic agents described above.

An "effective amount" of a polypeptide disclosed herein or an antagonist thereof, in reference to inhibition of neoplastic cell growth, tumor growth or cancer cell growth, is an amount capable of inhibiting to some extent, the growth of target cells. The term includes an amount capable of invoking a growth inhibitory, cytostatic and/or cytotoxic effect and/or apoptosis of the target cells. An "effective amount" of a LIV-1 polypeptide antagonist for purposes of inhibiting neoplastic cell growth, tumor growth or cancer cell (growth, may be determined empirically and in a routine manner.

A "therapeutically effective amount", in reference to the treatment of tumor, refers to an amount capable of invoking one or more of the following effects: (1) inhibition, to some extent, of tumor growth, including, slowing down and complete growth arrest; (2) reduction in the number of tumor cells; (3) reduction in tumor size; (4) inhibition (i.e., reduction, slowing down or complete stopping) of tumor cell infiltration into peripheral organs; (5) inhibition (i.e., reduction, slowing down or complete stopping) of metastasis; (6) enhancement of anti-tumor immune response, which may, but does not have to, result in the regression or rejection of the tumor; and/or (7) relief, to some extent, of one or more symptoms associated with the disorder. A "therapeutically effective amount" of a LIV-1 polypeptide antagonist for purposes of treatment of tumor may be determined empirically and in a routine manner.

A "growth inhibitory amount" of a LIV-1 antagonist is an amount capable of inhibiting the growth of a cell, especially tumor, e.g., cancer cell, either in vitro or in vivo. A "growth inhibitory amount" of a LIV-1 antagonist for purposes of inhibiting neoplastic cell growth may be determined empirically and in a routine manner.

A "cytotoxic amount" of a LIV-1 antagonist is an amount capable of causing the destruction of a cell, especially tumor, e.g., cancer cell, either in vitro or in vivo. A "cytotoxic amount" of a LIV-1 antagonist for purposes of inhibiting neoplastic cell growth may be determined empirically and in a routine manner.

"Percent (%) amino acid sequence homology or identity" with respect to the LIV-1 polypeptide sequences identified herein is defined as the percentage of amino acid residues in a candidate sequence that are identical with the amino acid residues in a LIV-1 sequence, after aligning the sequences and introducing gaps, if necessary, to achieve the maximum percent sequence identity, and not considering any conservative substitutions as part of the sequence identity. Alignment for purposes of determining percent amino acid sequence identity can be achieved in various ways that are within the skill in the art, for instance, using publicly available computer software such as BLAST, BLAST-2, ALIGN, ALIGN-2 or Megalign (DNASTAR) software. Those skilled in the art can determine appropriate parameters for measuring alignment, including any algorithms needed to achieve maximal alignment over the full-length of the sequences being compared. For purposes herein, however, % amino acid sequence identity values are obtained as described below by using the sequence comparison computer program ALIGN-2, wherein the complete source code for the ALIGN-2 program was authored by Genentech, Inc., and the source code shown in FIGS. 20A-Q has been filed with user documentation in the U.S. Copyright Office. Washington D.C., 20559, where it is registered under U.S. Copyright Registration No. TXU510087, and is provided in Table 1. The ALIGN-2 program is publicly available through Genentech, Inc. South San Francisco, Calif. The ALIGN-2 program should be compiled for use on a UNIX operating system, preferably digital UNIX V4.0D. All sequence comparison parameters are set by the ALIGN-2 program and do not vary.

For purposes herein, the % amino acid sequence identity of a given amino acid sequence A to, with, or against a given amino acid sequence B (which can alternatively be phrased as a given amino acid sequence A that has or comprises a certain % amino acid sequence identity to, with or against a given amino acid sequence B) is calculated as follows: 100 times the fraction X/Y where X is the number of amino acid residues scored as identical matches by the sequence alignment program ALIGN-2 in that program's alignment of A and B, and where Y is the total number of amino acid residues in B. It will be appreciated that where the length of amino acid sequence A is not equal to the length of amino acid sequence B, the % amino acid sequence identity of A to B will not equal the % amino acid sequence identity of B to A.

Unless specifically stated otherwise, all % amino acid sequence homology or identity values used herein are obtained as described above using the ALIGN-2 sequence comparison computer program. However, % amino acid sequence identity may also be determined using the sequence comparison program NCBI-BLAST2 (Altschul et al., Nucleic Acids Res., 25:3389-3402 (1997)). The NCBI-BLAST2 sequence comparison program may be downloaded from (www.)ncbi.nlm.nih.gov. NCBI-BLAST2 uses several search parameters, wherein all of those search parameters are set to default values including, for example, unmask=yes, strand=all, expected occurrences=10, minimum low complexity length=15/5, multi-pass e-value=0.01, constant for multi-pass=25, dropoff for final gapped alignment=25 and scoring matrix=BLOSUM62.

In situations where NCBI-BLAST2 is employed for amino acid sequence comparisons, the % amino acid sequence identity of a given amino acid sequence A to, with, or against a given amino acid sequence B (which can alternatively be phrased as a given amino acid sequence A that has or comprises a certain % amino acid sequence identity to, with, or against a given amino acid sequence B) is calculated as follows: 100 times the fraction X/Y where X is the number of amino acid residues scored as identical matches by the sequence alignment program NCBI-BLAST2 in that program's alignment of A and B, and where Y is the total number of amino acid residues in B. It will be appreciated that where the length of amino acid sequence A is not equal to the length of amino acid sequence B, the % amino acid sequence identity of A to B will not equal the % amino acid sequence identity of B to A.

In addition, % amino acid sequence identity may also be determined using the WU-BLAST-2 computer program (Altschul et al., Methods in Enzymology, 266:460-480 (1996)). Most of the WU-BLAST-2 search parameters are set to the default values. Those not set to default values, i.e., the adjustable parameters, are set with the following values: overlap span=1, overlap fraction=0.125, word threshold (T)=11, and scoring matrix=BLOSUM62. For purposes herein, a % amino acid sequence identity value is determined by dividing (a) the number of matching identical amino acids residues between the amino acid sequence of the LIV-1 polypeptide of interest having a sequence derived from the native LIV-1 polypeptide encoded by DNA 164647 and the comparison amino acid sequence of interest (i.e., the sequence against which the LIV-1 polypeptide of interest is being compared which may be a LIV-1 variant polypeptide) as determined by WU BLAST-2 by (b) the total number of amino acid residues of the LIV-1 polypeptide of interest. For example, in the statement "a polypeptide comprising an amino acid sequence A which has or having at least 80% amino acid sequence identity to the amino acid sequence B", the amino acid sequence A is the comparison amino acid sequence of interest and the amino acid sequence B is the amino acid sequence of the LIV-1 polypeptide of interest.

"Percent (%) nucleic acid sequence homology or identity" with respect to the LIV-1 polypeptide-encoding nucleic acid sequences identified herein is defined as the percentage of nucleotides in a candidate sequence that are identical with the nucleotides in a LIV-1 polypeptide-encoding nucleic acid sequence, after aligning the sequences and introducing gaps, if necessary, to achieve the maximum percent sequence identity. Alignment for purposes of determining percent nucleic acid sequence identity can be achieved in various ways that are within the skill in the art, for instance, using publicly available computer software such as BLAST, BLAST-2, ALIGN, ALIGN-2 or Megalign (DNASTAR) software. Those skilled in the art can determine appropriate parameters for measuring alignment, including any algorithms needed to achieve maximal alignment over the full-length of the sequences being compared. For purposes herein, however, % nucleic acid sequence identity values are obtained as described below by using the sequence comparison computer program ALIGN-2, wherein the complete source code for the ALIGN-2 program is has been filed with user documentation in the U.S. Copyright Office, Washington D.C., 20559, where it is registered under U.S. Copyright Registration No. TXU510087 and is provided herein in Table 1 as source code. The ALIGN-2 program is publicly available through Genentech, Inc., South San Francisco, Calif. The ALIGN-2 program should be compiled for use on a UNIX operating system, preferably digital UNIX V4.0D. All sequence comparison parameters are set by the ALIGN-2 program and do not vary

For purposes herein, the % nucleic acid sequence identity of a given nucleic acid sequence C to, with, or against a given nucleic acid sequence D (which can alternatively be phrased as a given nucleic acid sequence C that has or comprises a certain % nucleic acid sequence identity to with, or against a given nucleic acid sequence D) is calculated as follows: 100 times the fraction W/Z where W is the number of nucleotides scored as identical matches by the sequence alignment program ALIGN-2 in that program's alignment of C and D, and where Z is the total number of nucleotides in D. It will be appreciated that where the length of nucleic acid sequence C is not equal to the length of nucleic acid sequence D, the % nucleic acid sequence identity of C to D will not equal the % nucleic acid sequence identity of D to C.

Unless specifically stated otherwise, all % nucleic acid sequence identity values used herein are obtained as described above using the ALIGN-2 sequence comparison computer program. However, % nucleic acid sequence identity may also be determined using the sequence comparison program NCBI-BLAST2 (Altschul et al., Nucleic Acids Res., 25:3389-3402 (1997)). The NCBI-BLAST2 sequence comparison program may be downloaded from (www.)ncbi.nlm.nih.gov. NCBI-BLAST2 uses several search parameters, wherein all of those search parameters are set to default values including, for example, unmask=yes, strand=all, expected occurrences=10, minimum low complexity length=15/5, multi-pass e-value=0.01, constant for multi-pass=25, dropoff for final gapped alignment=25 and scoring matrix=BLOSUM62.

In situations where NCBI-BLAST2 is employed for sequence comparisons, the % nucleic acid sequence identity of a given nucleic acid sequence C to, with, or against a given nucleic acid sequence D (which can alternatively be phrased as a given nucleic acid sequence C that has or comprises a certain % nucleic acid sequence identity to, with, or against a given nucleic acid sequence D) is calculated as follows: 100 times the fraction W/Z where W is the number of nucleotides scored as identical matches by the sequence alignment program NCBI-BLAST2 in that program's alignment of C and D, and where Z is the total number of nucleotides in D. It will be appreciated that where the length of nucleic acid sequence C is not equal to the length of nucleic acid sequence D, the % nucleic acid sequence identity of C to D will not equal the % nucleic acid sequence identity of D to C.

In addition, % nucleic acid sequence identity values may also be generated using the WU-BLAST-2 computer program (Altschul et al., Methods in Enzymology, 266:460-480 (1996)). Most of the WU-BLAST-2 search parameters are set to the default values. Those not set to default values, i.e., the adjustable parameters, are set with the following values: overlap span=1, overlap fraction=0.125, word threshold (T)=11, and scoring matrix=BLOSUM62. For purposes herein, a % nucleic acid sequence identity value is determined by dividing (a) the number of matching identical nucleotides between the nucleic acid sequence of the LIV-1 polypeptide-encoding nucleic acid molecule of interest having a sequence derived from the native sequence LIV-1 polypeptide-encoding nucleic acid and the comparison nucleic acid molecule of interest (i.e., the sequence against which the LIV-1 polypeptide-encoding nucleic acid molecule of interest is being compared which may be a variant LIV-1 polynucleotide) as determined by WU-BLAST-2 by (b) the total number of nucleotides of the LIV-1 polypeptide-encoding nucleic acid molecule of interest. For example, in the statement "an isolated nucleic acid molecule comprising a nucleic acid sequence A which has or having at least 80% nucleic acid sequence identity to the nucleic acid sequence B", the nucleic acid sequence A is the comparison nucleic acid molecule of interest and the nucleic acid sequence B is the nucleic acid sequence of the LIV-1 polypeptide-encoding nucleic acid molecule of interest.

The term "positives", in the context of the amino acid sequence identity comparisons performed as described above, includes amino acid residues in the sequences compared that are not only identical, but also those that have similar properties. Amino acid residues that score a positive value to an amino acid residue of interest are those that are either identical to the amino acid residue of interest or are a preferred substitution (as defined in Table 2 below) of the amino acid residue of interest.

TABLE-US-00001 TABLE 2 Original Exemplary Preferred Residue Substitutions Substitutions Ala (A) val; leu; ile val Arg (R) lys; gln; asn lys Asn (N) gln: his; lys; arg gln Asp (D) glu glu Cys (C) ser ser Gln (Q) asn asn Glu (E) asp asp Gly (G) pro; ala ala His (H) asn; gln; lys; arg arg Ile (I) leu; val; met; ala; phe; leu norleucine Leu (L) norleucine: ile: val; ile met; ala; phe Lys (K) arg; gln; asn arg Met (M) leu; phe; ile leu Phe (F) leu; val; ile; ala; tyr leu Pro (P) ala ala Ser (S) thr thr Thr (T) ser ser Trp (W) tyr; phe tyr Tyr (Y) trp; phe; thr; ser phe Val (V) ile; leu; met; phe; leu ala; norleucine

Substantial modifications in function or immunological identity of the polypeptide are accomplished by selecting substitutions that differ significantly in their effect on maintaining (a) the structure of the polypeptide backbone in the area of the substitution, for example, as a sheet or helical conformation, (b) the charge or hydrophobicity of the molecule at the target site, or (c) the bulk of the side chain. Naturally occurring residues are divided into groups based on common side-chain properties: (1) hydrophobic: norleucine, met, ala, val, leu, ile; (2) neutral hydrophilic: cys, ser, thr; (3) acidic: asp, glu; (4) basic: asn, gln, his, lys, arg; (5) residues that influence chain orientation: gly, pro; and (6) aromatic: trp, tyr, phe.

Non-conservative substitutions will entail exchanging a member of one of these classes for another class. Such substituted residues also may be introduced into the conservative substitution sites or, more preferably, into the remaining (non-conserved) sites.

The variations can be made using methods known in the art such as oligonucleotide-mediated (site-directed) mutagenesis, alanine scanning, and PCR mutagenesis. Site-directed mutagenesis [Carter et al., Nucl. Acids Res., 13:4331 (1986), Zoller et al., Nucl. Acids Res. 10:6487 (1987)], cassette mutagenesis [Wells et al., Gene. 34:315 (1985)], restriction selection mutagenesis [Wells et al., Philos. Trans. R. Soc. London SerA, 317:415 (1986)] or other known techniques can be performed.

For purposes herein, the % value of positives of a given amino acid sequence A to, with, or against a given amino acid sequence B (which can alternatively be phrased as a given amino acid sequence A that has or comprises a certain % positives to, with, or against a given amino acid sequence B) is calculated as follows: 100 times the fraction X/Y where X is the number of amino acid residues scoring a positive value as defined above by the sequence alignment program ALIGN-2 in that program's alignment of A and B, and where Y is the total number of amino acid residues in B. It will be appreciated that where the length of amino acid sequence A is not equal to the length of amino acid sequence B, the % positives of A to B will not equal the % positives of B to A.

"Isolated." when used to describe the various polypeptides disclosed herein, means polypeptide that has been identified and separated and/or recovered from a component of its natural environment. Preferably, the isolated polypeptide is free of association with all components with which it is naturally associated. Contaminant components of its natural environment are materials that would typically interfere with diagnostic or therapeutic uses for the polypeptide, and may include enzymes, hormones, and other proteinaceous or non-proteinaceous solutes. In preferred embodiments, the polypeptide will be purified (1) to a degree sufficient to obtain at least 15 residues of N-terminal or internal amino acid sequence by use of a spinning cup sequenator, or (2) to homogeneity by SDS-PAGE under non-reducing or reducing conditions using Coomassie blue or, preferably, silver stain. Isolated polypeptide includes polypeptide in situ within recombinant cells, since at least one component of the LIV-1 natural environment will not be present. Ordinarily, however, isolated polypeptide will be prepared by at least one purification step.

An "isolated" nucleic acid molecule encoding a LIV-1 polypeptide or an "isolated" nucleic acid encoding an anti-LIV-1 antibody, is a nucleic acid molecule that is identified and separated from at least one contaminant nucleic acid molecule with which it is ordinarily associated in the natural source of the LIV-1-encoding nucleic acid or the anti-LIV-1-encoding nucleic acid. Preferably, the isolated nucleic acid is free of association with all components with which it is naturally associated. An isolated LIV-1-encoding nucleic acid molecule or an anti-LIV-1-encoding nucleic acid molecule is other than in the form or setting in which it is found in nature.

The term "control sequences" refers to DNA sequences necessary for the expression of an operably linked coding sequence in a particular host organism. The control sequences that are suitable for prokaryotes, for example, include a promoter, optionally an operator sequence, and a ribosome binding site. Eukaryotic cells are known to utilize promoters, polyadenylation signals, and enhancers.

Nucleic acid is "operably linked" when it is placed into a functional relationship with another nucleic acid sequence. For example, DNA for a presequence or secretory leader is operably linked to DNA for a polypeptide if it is expressed as a preprotein that participates in the secretion of the polypeptide; a promoter or enhancer is operably linked to a coding sequence if it affects the transcription of the sequence; or a ribosome binding site is operably linked to a coding sequence if it is positioned so as to facilitate translation. Generally, "operably linked" means that the DNA sequences being linked are contiguous, and, in the case of a secretory leader, contiguous and in reading phase. However, enhancers do not have to be contiguous. Linking is accomplished by ligation at convenient restriction sites. If such sites do not exist, the synthetic oligonucleotide adaptors or linkers are used in accordance with conventional practice.

"Stringency" of hybridization reactions is readily determinable by one of ordinary skill in the art, and generally is an empirical calculation dependent upon probe length, washing temperature, and salt concentration. In general, longer probes require higher temperatures for proper annealing, while shorter probes need lower temperatures. Hybridization generally depends on the ability of denatured DNA to reanneal when complementary strands are present in an environment below their melting temperature. The higher the degree of desired homology between the probe and hybridizable sequence, the higher the relative temperature which can be used. As a result, it follows that higher relative temperatures would tend to make the reaction conditions more stringent, while lower temperatures less so. For additional details and explanation of stringency of hybridization reactions, see Ausubel et al., Current Protocols in Molecular Biology, Wiley Interscience Publishers. (1995).

"Stringent conditions" or "high stringency conditions", as defined herein, may be identified by those that: (1) employ low ionic strength and high temperature for washing, for example 0.015 M sodium chloride/0.0015 M sodium citrate/0.1% sodium dodecyl sulfate at 50.degree. C.; (2) employ during hybridization a denaturing agent, such as formamide, for example, 50% (v/v) formamide with 0.1% bovine serum albumin/0.1% Ficoll/0.1% polyvinylpyrrolidone/50 mM sodium phosphate buffer at pH 6.5 with 750 mM sodium chloride, 75 mM sodium citrate at 42.degree. C.; or (3) employ 50% formamide, 5.times.SSC (0.75 M NaCl, 0.075 M sodium citrate). 50 mM sodium phosphate (pH 6.8), 0.1% sodium pyrophosphate, 5.times. Denhardt's solution, sonicated salmon sperm DNA (50 g/ml), 0.1% SDS, and 10% dextran sulfate at 42.degree. C., with washes at 42.degree. C. in 0.2.times.SSC (sodium chloride/sodium citrate) and 50% formamide at 55.degree. C., followed by a high-stringency wash consisting of 0.1.times.SSC containing EDTA at 55.degree. C.

"Moderately stringent conditions" may be identified as described by Sambrook et al., Molecular Cloning: A Laboratory Manual, New York: Cold Spring Harbor Press, 1989, and include the use of washing solution and hybridization conditions (e.g., temperature, ionic strength and % SDS) less stringent than those described above. An example of moderately stringent conditions is overnight incubation at 37.degree. C. in a solution comprising 20% formamide, 5.times.SSC (150 mM NaCl, 15 mM trisodium citrate), 50 mM sodium phosphate (pH 7.6), 5.times. Denhardt's solution, 10% dextran sulfate, and 20 mg/ml denatured sheared salmon sperm DNA, followed by washing the filters in 1.times.SSC at about 35-50.degree. C. The skilled artisan will recognize how to adjust the temperature, ionic strength, etc. as necessary to accommodate factors such as probe length and the like.

"Active" or "activity" for the purposes herein refers to form(s) of LIV-1 polypeptides which retain a biological and/or an immunological activity/property of a native or naturally-occurring LIV-1 polypeptide, wherein "biological" activity refers to a function (either inhibitory or stimulatory) caused by a native or naturally-occurring LIV-1 polypeptide other than the ability to induce the production of an antibody against an antigenic epitope possessed by a a native or naturally-occurring LIV-1 polypeptide and an "immunological" activity refers to the ability to induce the production of an antibody against an antigenic epitope possessed by a native or naturally-occurring LIV-1 polypeptide.

"Biological activity" in the context of an antibody or another antagonist molecule that can be identified by the screening assays disclosed herein (e.g., an organic or inorganic small molecule, peptide, etc.) is used to refer to the ability of such molecules to bind or complex with the polypeptides encoded by the amplified genes identified herein, or otherwise interfere with the interaction of the encoded polypeptides with other cellular proteins or otherwise interfere with the transcription or translation of a LIV-1 polypeptide. A preferred biological activity is growth inhibition of a target tumor cell. Another preferred biological activity is cytotoxic activity resulting in the death of the target tumor cell.

The term "biological activity" in the context of a LIV-1 polypeptide means the ability of a LIV-1 polypeptide to induce neoplastic cell growth or uncontrolled cell growth or to act as an indication of a particular form of neoplasm that is particularly metastatic.

The phrase "immunological activity" means immunological cross-reactivity with at least one epitope of a LIV-1 polypeptide.

"Immunological cross-reactivity" as used herein means that the candidate polypeptide is capable of competitively inhibiting the qualitative biological activity of a LIV-1 polypeptide having this activity with polyclonal antisera raised against the known active LIV-1 polypeptide. Such antisera are prepared in conventional fashion by injecting goats or rabbits, for example, subcutaneously with the known active analogue in complete Freund's adjuvant, followed by booster intraperitoneal or subcutaneous injection in incomplete Freunds. The immunological cross-reactivity preferably is "specific", which means that the binding affinity of the immunologically cross-reactive molecule (e.g. antibody) identified, to the corresponding LIV-1 polypeptide is significantly higher (preferably at least about 2-times, more preferably at least about 4-times, even more preferably at least about 8-times, most preferably at least about 10-times higher) than the binding affinity of that molecule to any other known native polypeptide.

The term "antagonist" is used in the broadest sense, and includes any molecule that partially or fully blocks, inhibits, or neutralizes a biological activity of a native LIV-1 polypeptide disclosed herein or the transcription or translation thereof. Suitable antagonist molecules specifically include antagonist antibodies or antibody fragments, fragments, peptides, small organic molecules, anti-sense nucleic acids, etc. Included are methods for identifying antagonists of a LIV-1 polypeptide with a candidate antagonist molecule and measuring a detectable chance in one or more biological activities normally associated with the LIV-1 polypeptide.

A "small molecule" is defined herein to have a molecular weight below about 500 Daltons.

The word "label" when used herein refers to a detectable compound or composition which is conjugated directly or indirectly to the antibody so as to generate a "labeled" antibody. The label may be detectable by itself (e.g., radioisotope labels or fluorescent labels) or, in the case of an enzymatic label, may catalyze chemical alteration of a substrate compound or composition which is detectable. Radionuclides that can serve as detectable labels include, for example, I-131, I-123, I-125, Y-90, Re-188, Re-186, At-211, Cu-67, Bi-212, and Pd109.

By "solid phase" is meant a non-aqueous matrix to which the antibody of the present invention can adhere. Examples of solid phases encompassed herein include those formed partially or entirely of glass (e.g., controlled pore glass), polysaccharides (e.g., agarose), polyacrylamides, polystyrene, polyvinyl alcohol and silicones. In certain embodiments, depending on the context, the solid phase can comprise the well of an assay plate: in others it is a purification column (e.g., an affinity chromatography column). This term also includes a discontinuous solid phase of discrete particles, such as those described in U.S. Pat. No. 4,275,149.

A "liposome" is a small vesicle composed of various types of lipids, phospholipids and/or surfactant which is useful for delivery of a drug (such as a LIV-1 polypeptide or antibody thereto and, optionally, a chemotherapeutic agent) to a mammal. The components of the liposome are commonly arranged in a bilayer formation, similar to the lipid arrangement of biological membranes.

As used herein, the term "immunoadhesin" designates antibody-like molecules which combine the binding specificity of a heterologous protein (an "adhesin," for example a receptor, ligand, or enzyme) with the effector functions of immunoglobulin constant domains. Structurally, the immunoadhesins comprise a fusion of the adhesin amino acid sequence with the desired binding specificity which is other than the antigen recognition and binding site (antigen combining site) of an antibody (i.e., is "heterologrous"), and an immunoglobulin constant domain sequence. The adhesin part of an immunoadhesin molecule typically is a continuous amino acid sequence comprising at least the binding site of a receptor or a ligand. The immunoglobulin constant domain sequence in the immunoadhesin may be obtained from any immunoglobulin, such as IgG-1, IgG-2, IgG-3, or IgG-4 subtypes. IgA (including IgA-1 and IgA-2), IgE, IgD or IgM, and any subclass or isotype thereof.

The terms "HER2", "ErbB2" "c-Erb-B2" are used interchangeably. Unless indicated otherwise, the terms "ErbB2" "c-Erb-B2" and "HER2" when used herein refer to the human protein, and "erbB2,", "c-erb-B2," and "her2" refer to human gene. The human erbB2 gene and ErbB2 protein are, for example, described in Semba et al., PNAS (USA) 82:6497-6501 (1985) and Yamamoto et al., Nature 319:230-234 (1986)(Genebank accession number X03363). ErbB2 comprises four domains (Domains 1-4).

The "epitope 4D5" is the region in the extracellular domain of ErbB2 to which the antibody 4D5 (ATCC CRL 10463) binds. This epitope is close to the transmembrane region of ErbB2. To screen for antibodies which bind to the 4D5 epitope, a routine cross-blocking assay such as that described in Antibodies, A Laboratory Manual, Cold Spring Harbor Laboratory, Ed Harlow and David Lane (1988), can be performed. Alternatively, epitope mapping can be performed to assess whether the antibody binds to the 4D5 epitope of ErbB2 (i.e. any one or more residues in the region from about residue 529, e.g. about residue 561 to about residue 625, inclusive).

The "epitope 3H4" is the region in the extracellular domain of ErbB2 to which the antibody 3H4 binds. This epitope includes residues from about 541 to about 599, inclusive, in the amino acid sequence of ErbB2 extracellular domain.

The "epitope 7C2/7F3" is the region at the N terminus of the extracellular domain of ErbB2 to which the 7C2 and/or 7F3 antibodies (ATCC HB-12215 and ATCC HB-12216, respectively) bind. To screen for antibodies which bind to the 7C2/7F3 epitope, a routine cross-blocking assay such as that described in Antibodies, A Laboratory Manual, Cold Spring Harbor Laboratory, Ed Harlow and David Lane (1988), can be performed. Alternatively, epitope mapping can be performed to establish whether the antibody binds to the 7C2/7F3 epitope on ErbB2.

The term "induces cell death" or "capable of inducing cell death" refers to the ability of the anti-LIV-1 gene product antibody, alone or in co-treatment with a chemotherapeutic agent, to make a viable cell become nonviable. The "cell" here is one which expresses the LIV-1 gene product, especially where the cell overexpresses the LIV-1 gene product. A cell which "overexpresses" LIV-1 has significantly higher than normal LIV-1 mRNA and/or LIV-1 protein levels compared to a noncancerous cell of the same tissue type. A cell to be treated by the method of the invention does not also overexpress ErbB2 (i.e. the cell expresses ErbB2 at a level that is approximately the same or less than a normal, non-cancerous cell of the same cell or tissue type). Preferably, the cell is a cancer cell, e.g. a breast, lung, or prostate cell, In vitro, the cell may be from a cell line transformed with LIV-1 DNA, preferably DNA 164647, to express LIV-1 on the cell surface. Cell death in vitro may be determined in the absence of complement and immune effector cells to distinguish cell death induced by antibody dependent cellular cytotoxicity (ADCC) or complement dependent cytotoxicity (CDC). Thus, the assay for cell death may be performed using heat inactivated serum (i.e. in the absence of complement) and in the absence of immune effector cells. To determine whether the antibody is able to induce cell death, loss of membrane integrity as evaluated by uptake of propidium iodide (PI), trypan blue (see Moore et al., Cytotechnology 17:1-11 [1995]) or 7AAD can be assessed relative to untreated cells. Preferred cell death-inducing antibodies are those which induce PI uptake in the "PI uptake assay in LIV-1 expressing cells".

The phrase "induces apoptosis" or "capable of inducing apoptosis" refers to the ability of the antibody to induce programmed cell death as determined by binding of annexin V, fragmentation of DNA, cell shrinkage, dilation of endoplasmic reticulum, cell fragmentation, and/or formation of membrane vesicles (called apoptotic bodies). The cell is one which overexpresses the LIV-1 gene product. Preferably the "cell" is a tumor cell, e.g. a breast, lung, or prostate cell. In vitro, the cell may be from a cell line transformed with LIV-1 DNA, such as DNA 164647. Various methods are available for evaluating the cellular events associated with apoptosis. For example, phosphatidyl serine (PS) translocation can be measured by annexin binding; DNA fragmentation can be evaluated through DNA laddering as disclosed in the example herein; and nuclear/chromatin condensation along with DNA fragmentation can be evaluated by any increase in hypodiploid cells. Preferably, the antibody which induces apoptosis is one which results in about 2 to 50 fold, preferably about 5 to 50 fold, and most preferably about 10 to 50 fold induction of annexin binding relative to untreated cell in an "annexin binding assay using cells" (see below).

As used herein, the term "salvage receptor binding epitope" refers to an epitope of the Fc region of an IgG molecule (e.g., IgG.sub.1, IgG.sub.2, IgG.sub.3, or IgG.sub.4) that is responsible for increasing the in vitro serum half-life of the IgG molecule.

"Treatment" refers to both therapeutic treatment and prophylactic or preventative measures. Those in need of treatment include those already with the disorder as well as those in which the disorder is to be prevented.

A "disorder" is any condition that would benefit from treatment with the anti-LIV-1 gene product antibody. This includes chronic and acute disorders or diseases including those pathological conditions which predispose the mammal to the disorder in question. Non-limiting examples of disorders to be treated herein include benign and malignant tumors of breast, lung, and prostate tissue.

The term "package insert" is used to refer to instructions customarily included in commercial packages of therapeutic products, that contain information about the indications, usage, dosage, administration, contraindications and/or warnings concerning the use of such therapeutic products.

The term "serum concentration," "serum drug concentration," or serum anti-LIV-1 "antibody concentration" refers to the concentration of a drug in the blood serum of an animal or human patient being treated with the drugs. Serum concentration of antibody, for example, is preferably determined by immunoassay. Preferably, the immunoassay is ELISA according to the procedure disclosed herein.

The term "peak serum concentration" refers to the maximal serum drug concentration shortly after delivery of the drug into the animal or human patient, after the drug has been distributed throughout the blood system, but before significant tissue distribution, metabolism or excretion of drug by the body has occurred.

The term "trough serum concentration" refers to the serum drug concentration at a time after delivery of a previous dose and immediately prior to delivery of the next subsequent dose of drug in a series of doses. Generally, the trough serum concentration is a minimum sustained efficacious drug concentration in the series of drug administrations. Also, the trough serum concentration is frequently targeted as a minimum serum concentration for efficacy because it represents the serum concentration at which another dose of drug is to be administered as part of the treatment regimen. If the delivery of drug is by intravenous administration, the trough serum concentration is most preferably attained within 1 day of a front loading initial drug delivery. It the delivery of drug is by subcutaneous administration, the peak serum concentration is preferably attained in 3 days or less. According to the invention, the trough serum concentration is preferably attained in 4 weeks or less, preferably 3 weeks or less, more preferably 2 weeks or less, most preferably in 1 week or less, including 1 day or less using any of the drug delivery methods disclosed herein.

The term "intravenous infusion" refers to introduction of a drug into the vein of an animal or human patient over a period of time greater than approximately 5 minutes, preferably between approximately 30 to 90 minutes, although, according to the invention, intravenous infusion is alternatively administered for 10 hours or less.

The term "intravenous bolus" or "intravenous push" refers to drug administration into a vein of an animal or human such that the body receives the drug in approximately 15 minutes or less, preferably 5 minutes or less.

The term "subcutaneous administration" refers to introduction of a drug under the skin of an animal or human patient, preferable within a pocket between the skin and underlying tissue, by relatively slow, sustained delivery from a drug receptacle. The pocket may be created by pinching or drawing the skin up and away from underlying tissue.

The term "subcutaneous infusion" refers to introduction of a drug under the skin of an animal or human patient, preferably within a pocket between the skin and underlying tissue, by relatively slow, sustained delivery from a drug receptacle for a period of time including, but not limited to, 30 minutes or less, or 90 minutes or less. Optionally, the infusion may be made by subcutaneous implantation of a drug deliver, pump implanted under the skin of the animal or human patient, wherein the pump delivers a predetermined amount of drug for a predetermined period of time, such as 30 minutes, 90 minutes, or a time period spanning the length of the treatment regimen.

The term "subcutaneous bolus" refers to drug administration beneath the skin of an animal or human patient, where bolus drug delivery is preferably less than approximately 15 minutes, more preferably less than 5 minutes, and most preferably less than 60 seconds. Administration is preferably within a pocket between the skin and underlying tissue, where the pocket is created, for example, by pinching or drawing the skin up and away from underlying tissue.

The term "front loading," when referring to drug administration is meant to describe an initially higher dose followed by the same or lower doses at intervals. The initial higher dose or doses are meant to more rapidly increase the animal or human patient's serum drug concentration to an efficacious target serum concentration.

Published information related to LIV-1 gene expression and gene product includes the following issued patents and published applications: Manning, D. L. et al., U.S. Pat. No. 5,693,465, issued Dec. 2, 1997; Manning, D. L. et al., European J. Cancer 29A(10):1462-1468 [1993]; Manning, D. L. et al., European J. Cancer, 30A(5):675-678 [1994]; Manning. D. L. et al., Acta Oncologica 34(5):641-646 [1995]; McClelland, R. A. et al., Breast Cancer Res. & Treatment 41(1):31-41 [1996]; Knowlden, J. M. et al. Clin. Cancer Res. 3(11):2165-2172 [1997]; and McClelland, R. A. et al., British J. Cancer 77(10):1653-1656 [1998].

Published information related to anti-ErbB2 antibody includes the following issued patents and published applications: PCT/US89/00051, published Jan. 5, 1989, PCT/US90/02697, published May 18, 1990, EU 0474727, issued Jul. 23, 1997, DE 69031120.6, issued Jul. 23, 1997, PCT/US97/18385, published Oct. 9, 1997, SA 97/9185, issued Oct. 14, 1997, U.S. Pat. No. 5,677,171, issued Oct. 14, 1997, U.S. Pat. No. 5,720,937, issued Feb. 24, 1998. U.S. Pat. No. 5,720,954, issued Feb. 24, 1998, U.S. Pat. No. 5,725,856, issued Mar. 10, 1998, U.S. Pat. No. 5,770,195, issued Jun. 23, 1998, U.S. Pat. No. 5,772,997, issued Jun. 30, 1998, PCT/US98/2626, published Dec. 10, 1998, and PCT/US99/06673, published Mar. 26, 1999, each of which patents and publications is herein incorporated by reference in its entirety.

The following examples are offered for illustrative purposes only, and are not intended to limit the scope of the present invention in any way.

All patent and literature references cited in the present specification are hereby incorporated by reference in their entirety.

EXAMPLES

Commercially available reagents referred to in the examples were used according to manufacturer's instructions unless otherwise indicated. The source of those cells identified in the following examples, and throughout the specification, by ATCC accession numbers is the American Type Culture Collection, Manassas, Va. Unless otherwise noted, the present invention uses standard procedures of recombinant DNA technology, such as those described herein and in the following textbooks: Sambrook et al., Molecular Cloning: A Laboratory Manual, Cold Spring Harbor Press N.Y. 1989; Ausubel et al., Current Protocols in Molecular Biology, Green Publishing Associates and Wiley Interscience, N.Y. 1989; Innis et al., PCR Protocols: A Guide to Methods and Applications, Academic Press, inc., N.Y. 1990; Harlow et al., Antibodies: A Laboratory Manual, Cold Spring Harbor Press, Cold Spring Harbor, 1988; Gait, M. J. Oligonucleotide Synthesis, IRL Press, Oxford, 1984, R. I. Freshney, Animal Cell Culture, 1987 Coligan et al., Current Protocols in Immunology, 1991.

Example 1

LIV-1 Expression in Tumor Cells Examined by Microarray Analysis

A form of breast cancer in which the cells overexpress the LIV-1 gene product (e.g. LIV-1-164647 mRNA) but do not overexpress ErbB2 has been discovered and is uniquely disclosed herein. Detection of the tumor type was made using microarray technology. Using nucleic acid microarrays, test and control mRNA samples from test and control tissue samples are reverse transcribed and labeled to generate cDNA probes. The cDNA probes are then hybridized to an array of nucleic acids immobilized on a solid support. The array is configured such that the sequence and position of each member of the array is known. Hybridization of a labeled probe with a particular array member indicates that the sample from which the probe was derived expresses that gene. If the hybridization signal of a probe from a test (disease tissue) sample is greater than hybridization signal of a probe from a control (normal tissue) sample, the gene or genes overexpressed in the disease tissue are identified. The implication of this result is that an overexpressed protein in a diseased tissue is useful not only as a diagnostic marker for the presence of the disease condition, but also as a therapeutic target for treatment of the disease condition.

Tumor cells were crossly dissected from surrounding, non-cancerous cells in breast tumor tissue. Hematoxylin and eosin staining of the cells confirmed that the excised cells were from tumor. The mRNA of the tumor cells (reflecting cell-specific expression of a variety of genes) was converted to cDNA by RT/PCR methodology, labeled with fluorescent tags, and allowed to hybridize to the ESTs arrayed on a class slide. An imaging device detected and measured the fluorescence of each sample on the slide, where fluorescence represents a labeled messenger from the test cells identifiable due to its hybridization with a known nucleic acid sequence (an EST) at a known position on the slide. Relative fluorescence indicated relative activity of a gene, with strong flourescence indicating an active gene expressing a relative large amount of messenger. Little or no flourescence indicated that no labeled messenger hybridized to the ESTs. Detection of fluorescently labeled probes hybridized to sequences on the microarray slide is described, for example, in U.S. Pat. No. 5,143,854, herein incorporated by reference.

It was found that cDNA of the preparation hybridized to a publicly available EST sequence (accession no. H29315 (from the Washington University-Merck EST Project, authors Hillier. L. et al., SEQ ID NO:5, purchased from Research Genetics (Alabama, USA) in a pattern suggesting overexpression in breast tumor tissue that did not also overexpress ErbB2. The cDNA was sequenced and disclosed herein as LIV-1-DNA 164647. In situ hybridization of a radioactivel